10 Timer balls
Buy 10 Timer Balls. These can be obtained from Rustboro City Poke Mart.
Go to the Cave of Origin in Sootopolis City. Have at least level 35 to 45 Pokémon, preferably with high hit points.
Go inside. Wander your way to Groudon (Level 45) and your Red Orb will start to glow. This will cause Groudon to walk toward you.
Groudon's moves are Bulk up, Fire Blast, Slash, and Earthquake. Send out a Flying-type first and stall the Groudon. The Timer Balls' catch rate doesn't go up if the Pokémon is weak, just if a lot of turns have been taken, so the more you stall, the better chance you have at catching it.
Eventually after a decent amount of turns, you should catch him with one of your timer balls.
Quick ball
Get a Quick Ball and loads of Timer Balls.
Get some Pokémon with no weakness to his moveset and high hp.
Find Groudon. Start battle. His standard moveset = Earthquake, Fire Blast, Solarbeam, Slash.
Throw Quick Ball on the first turn.
If it doesn't work, wait 10+ turns, then start throwing Timer Balls. If you run out, revert to the previous save.
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